S.M. Stoller Corporation
Environmental Surveillance, Education and Research Program
ISSN NUMBER 1089-5469
Idaho National Engineering and Environmental Laboratory Offsite Environmental
Surveillance Program Report:
Second Quarter 2003
September 2003

Contributors:
Marilyn Case, Christopher Martin
Program conducted for the U.S. Department of Energy, Idaho Operations Office
Under Contract DE-AC07-00ID13658
By the S.M. Stoller Corporation,
Environmental Surveillance, Education and Research Program
Douglas K. Halford, Program Manager
1780 First Street, Idaho Falls, Idaho 83401
www.stoller-eser.com
|
None of the radionuclides detected in any of the samples collected during the second quarter of 2003 could be directly linked with INEEL activities. Levels of detected radionuclides were no different than values measured at other locations across the United States or were consistent with levels measured historically at the INEEL. All detected radionuclide concentrations were well below guidelines set by the U.S. Department of Energy (DOE) and regulatory standards established by the U.S. Environmental Protection Agency (EPA) for protection of the public. (See Table E-1.) |
This report for the second quarter, 2003, contains results from the Environmental Surveillance, Education and Research (ESER) Program’s monitoring of the Department of Energy’s Idaho National Engineering and Environmental Laboratory’s (INEEL) offsite environment, April 1 through May 30, 2003. All sample types (media) and the sampling schedule followed during 2003 are listed in Appendix A. Specifically, this report contains the results for the following:
Air sampling, including air filters and charcoal cartridges, atmospheric moisture, and 10 micron particulate matter (PM10);
Water sampling, including precipitation, surface water, and drinking water;
Agricultural product sampling, including milk, sheep, and large game;
Measurement of external exposure, using environmental dosimetry.
Results are presented in this report with an analytical uncertainty term, s, where “s” is an estimate of the population standard deviation (s), assuming a normal (Guassian) distribution. The following guidelines, based on Currie (1984), are used to interpret the analytical results.
Results greater than 3s are reported as “detected”.
Results less than 2s are reported as “undetected”.
Results between 2-3s are reported as “questionable” (i.e., the radionuclide might have been detected but such detection may not be considered reliable.)
Gross alpha and gross beta measurements are used as general indicators of the presence of radionuclides. Gross alpha and gross beta results were found to have no discernable statistical distribution during the second quarter of 2003. Because of this, these data were statistically analyzed using nonparametric methods, including the use of the median to represent central tendency. At no time during the second quarter were weekly, monthly, or quarterly gross alpha or gross beta concentrations in air collected at Boundary locations statistically greater than corresponding data for Distant locations, as one would expect if the INEEL were a significant source of radionuclide contamination.
Iodine-131 (131I) was not detected in any batch of charcoal cartridges during the second quarter.
Selected quarterly composite filter samples were analyzed for gamma emitting radionuclides, strontium-90 (90Sr), plutonium-238 (238Pu), plutonium-239/240 (239/240Pu), and americium-241 (241Am). None of these radionuclides were detected in any sample collected and composited during the second quarter.
Twelve atmospheric moisture samples were obtained during the second quarter of 2003; two each from Atomic City and Blackfoot, three from Rexburg, and five from Idaho Falls. None of the exceeded their respective 3s levels.
The ESER Program operates three PM10 samplers, one each at Rexburg, Blackfoot, and Atomic City. Sampling of PM10 is informational as no analyses are conducted for contaminants. PM10 concentrations were well below all health standard levels for all samples. The maximum 24-hour concentration was 73.04 mg/m3 on June 19, 2003, at Atomic City. This below the EPA Air Quality Standard of 150 mg/m3.
Sufficient precipitation occurred to allow collection of three monthly composite samples from Idaho Falls, two monthly composite samples from the Central Facilities Area (CFA) on the INEEL, and eight weekly samples from the Experimental Field Station (EFS) on the INEEL. Tritium was not detected above the 3s level in any of the samples.
Thirteen drinking water samples and one duplicate were collected from selected taps throughout southeast Idaho during the second quarter 2003. Samples were analyzed for gross alpha, gross beta, and tritium (3H). None of the samples exceeded its 3s value for gross alpha or tritium. Ten samples exceeded the 3s value for gross beta. The maximum gross beta concentration measured, (9.72 ± 0.17) pCi/L, was from Monteview and was below the EPA Safe Water Drinking Water Act (SDWA) screening limit of 50 pCi/L and the DOE DCG of 100 pCi/L. Levels of gross beta activity observed are not unusual given the basaltic terrain.
Six surface water samples (including one duplicate) were collected from locations throughout southeast Idaho. Samples were analyzed for gross alpha, gross beta, and tritium (3H). None of the samples exceeded its 3s value for tritium. Gross alpha and gross beta activities were detected in three and four samples, respectively. Results were less that SDWA screening limits and DOE DCGs and were typical of historical and regional measurements.
Milk samples were collected weekly in Idaho Falls and monthly at eight other locations around the INEEL. All samples were analyzed for gamma-emitting radionuclides. Iodine 131 and 137Cs concentrations were not detected in any milk sample.
Individual sheep from three separate flocks were sampled including a control flock in Dubois from the Experimental Sheep Station, a flock from a southern INEEL allotment, and a flock from a northern INEEL allotment. Two sheep were taken from each flock. Thyroid, muscle, and liver tissue were collected and analyzed for gamma emitting radionuclides. No 131I was found in any of the samples. Analysis for 137Cs showed results greater than 3s in three samples from two different animals on the northern allotment: one liver and two muscle samples. All concentrations of 137Cs were similar to those found in both onsite and offsite sheep samples during recent years.
Two large game animals (a mule deer and a pronghorn) were sampled during the second quarter of 2003. They were killed as a result of a vehicular collision. Thyroid, liver, and muscle tissues were sampled. Only the naturally occurring radionuclide potassium-40 was measured at concentrations greater than the associated 3s uncertainty values. No human-made radionuclides were detected.
Environmental dosimeter locations are also divided into Boundary and Distant groupings. Boundary exposure rates ranged from a low of 0.28 mR/day to 0.34 mR/day. The overall Boundary average was 0.31 mR/day. The Distant group ranged from 0.25 mR/day to 0.38 mR/day, with an overall average exposure also of 0.31 mR/day. No statistical difference existed between Boundary and Distant locations. All exposure results are consistent with those measured historically.
Quality assurance samples submitted for analysis during the first quarter 2003 demonstrate that the results were reasonably complete, accurate, precise, and free of field contamination, as measured by criteria established in the ESER Quality Assurance Project Plan.
No radionuclide in any of
the samples taken during the second quarter of 2003 could be directly linked
with INEEL activities. Levels of detected radionuclides were no different than
values measured at other locations across the United States and consistent with
levels measured in the past in this area. Radionuclide concentrations in all of
the samples collected and analyzed during the second quarter, 2003 were below
guidelines set by both the DOE and the U.S. Environmental Protection Agency
(EPA) for protection of the public.
Table E-1 Summary
of results for the first quarter of 2003.
|
Media |
Sample Type |
Analysis |
Results |
|
Air |
Filters |
Gross alpha, gross beta |
There were no statistical differences noted for weekly, monthly or quarterly gross alpha or gross beta concentrations measured at INEEL, Boundary, and Distant locations. No result exceeded the DCG for gross alpha or gross beta activity in air. |
|
|
|
Gamma-emitting radionuclides, select actinides, 90Sr |
Gamma-emitting radionuclides, 241Am, 239/240Pu and 90Sr were not detected in any composite sample. |
|
|
Charcoal Cartridge |
Iodine-131 |
No detections of 131I were made during the second quarter. |
|
|
PM10 |
Particulate matter |
Forty-three total samples were collected from three locations. No regulatory limits were exceeded. |
|
Atmospheric Moisture |
Liquid |
Tritium |
Thirteen atmospheric moisture samples were collected. None of the results were greater than the 3s uncertainty. |
|
Precipitation |
Liquid |
Tritium |
No measurable concentrations of tritium were recorded during the second quarter. |
|
Drinking Water |
Liquid |
Gross alpha, gross beta, tritium |
Gross alpha activity was not detected in any sample. Gross beta activity was measured in 10 of 14 samples. The maximum was well below the EPA Safe Drinking Water Act limits. Tritium was not detected in any sample. at concentrations many times lower than the EPA screening level. |
|
Surface Water |
Liquid |
Gross alpha, gross beta, tritium |
No tritium was detected in any of the six samples collected. Gross alpha activity was measured in three samples at values greater than 3s. Gross beta activity was measured above the 3s values in four samples. All concentrations were below EPA and DOE limits, and ere within historical measurements. |
|
Milk |
Liquid |
Iodine-131, gamma emitting radionuclides |
No radionuclides were detected in any of samples collected. |
|
Sheep |
Tissue |
Iodine-131, gamma emitting radionuclides |
Cesium-137 was detected in three samples: two muscle samples and one liver from two sheep collected from the Northern allotment animal. |
|
Game Animals |
Tissue |
Iodine-131, gamma emitting radionuclides |
Two game animals were collected during this quarter. No man-made radionuclides were detected. |
|
Environmental Radiation |
TLD |
Ambient ionizing radiation |
Values were consistent with expected exposures given the altitude and location of the TLD's. There were no statistical differences between Boundary and Distant location results. |